Just spent 15 minutes trying to figure out how to remove accounts from Insync and still can’t find it. The “Remove account” button shown in another answer is missing. I got the latest app version 3.8.7.50516-jammy on Ubuntu.
That worked for me. I was able to delete accounts which had expired trials, on my Windows machine.
But the UX problem is that the icons are faded, i.e. not high contrast to their background, so they look “greyed-out”/“grayed-out” which implies that they are disabled, when actually they are not. So it misled me into thinking I couldn’t click them.